If you're an EU citizen then you have the right to live and work in Spain, but being fluent in Spanish is essential to get a job. Unemployment is incredibly high and jobs will go to Spaniards first.
However, if you're a non-EU citizen eg from Canada, USA, Australia, then it's actually illegal for you to move to Spain to live and work.
I would try Madrid or the Basque country as that's where the jobs are. I did not find Madrid very liveable. It all depends on your skills.
You wouldn't be able to move there without a job offer FIRST.
I'm in the works to plan a move and start a new life in Spain. Start fresh. I know the expenses will be there, but that aside, I'm looking for suggestions on which city and area in Spain is most livable, and have a good change of finding employment. Any suggestions?
